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Journal Articles

Chapter 7, Research and development and international cooperation on nuclear non-proliferation and nuclear security

Tomikawa, Hirofumi; Koizumi, Mitsuo; Tamai, Hiroshi

Genshiryoku Heiwa Riyo To Kakufukakusan, Kakusekyuritei; NSA/Commentaries, No.25, p.167 - 174, 2020/06

Japan's efforts for research and development on nuclear material detection and nuclear forensics and international cooperation are introduced focusing on the various aspects implemented in JAEA.

Journal Articles

Uranium age-dating using in-situ isotope ratios by thermal ionization mass spectrometry for nuclear forensics

Okubo, Ayako; Shinohara, Nobuo; Magara, Masaaki

Journal of Radioanalytical and Nuclear Chemistry, 314(1), p.231 - 234, 2017/10

 Times Cited Count:2 Percentile:19.65(Chemistry, Analytical)

The model date of two enriched uranium materials were determined using a new method for nuclear forensics investigation. In this method, the $$^{230}$$Th/$$^{234}$$U ratio was calculated without spike addition from measured ratios of $$^{230}$$Th/$$^{234}$$Th and $$^{234}$$U/$$^{238}$$U, and calculated $$^{234}$$Th/$$^{238}$$U ratio in secular equilibrium. The obtained model date for the low-enriched uranium material was agreed with the known production date within uncertainty. For the highly enriched uranium material, slightly younger model date than the known production date was obtained. The $$^{234}$$U interference on $$^{234}$$Th counting in thermal ionization mass spectrometry measurement was suspected as a potential cause.

Journal Articles

Prospective features for integration of nuclear forensics capability in national framework

Tamai, Hiroshi; Okubo, Ayako; Kimura, Yoshiki; Shinohara, Nobuo; Tazaki, Makiko; Shimizu, Ryo; Suda, Kazunori; Tomikawa, Hirofumi

Proceedings of INMM 58th Annual Meeting (Internet), 6 Pages, 2017/07

Nuclear forensics is a technical measure to analyse and collate samples of illegally used nuclear materials, etc., to clarify their origins, routes, etc. and contribute to criminal identifications. Close collaboration with police and judicial organizations is essential. The national response framework is being built up with international cooperation. Discussions on promoting technical capability and regional cooperation are presented.

Journal Articles

Prospects and challenges of the post-nuclear security summit phase

Tamai, Hiroshi

Hiroshima Repoto 2017-Nen Ban; Kakugunshuku, Kakufukakusan, Kakusekyuritei O Meguru 2016-Nen No Doko, p.163 - 165, 2017/03

The series of Nuclear Security Summit, initiated by President Barack Obama, was held biennially, four times since 2010, and played an important role in promoting international efforts to enhance nuclear security. Despite Russia's refusal to participate in the fourth meeting, these summit-level meetings have gained both international and domestic attention, which have led to remarkable improvements in the field of nuclear security of each participating country. Therefore, there is an urgent need to take continuous measures to keep this momentum alive even after the final Nuclear Security Summit concluded in 2016. The challenges in strengthening nuclear security, prospects in the post-Nuclear Security Summit phase, as well as efforts and measures that Japan should pursue are investigated.

Journal Articles

Technical/institutional prerequisite for nuclear forensics response framework

Tamai, Hiroshi; Okubo, Ayako; Kimura, Yoshiki; Kokaji, Lisa; Shinohara, Nobuo; Tomikawa, Hirofumi

Dai-37-Kai Kaku Busshitsu Kanri Gakkai Nihon Shibu Nenji Taikai Rombunshu (CD-ROM), 8 Pages, 2017/02

Nuclear Forensics capability has been developed under the international collaborations. For its effective function, technical development in analysis of seized nuclear materials as well as the institutional development in comprehensive response framework are required under individual national responsibility. In order to keep the "chain of custody" in the proper operation of sample collection at the event scene, radiological analysis at the laboratory, storage of the samples, and further inspection and trial, close cooperation and information sharing between relevant organisations are essential. IAEA issues the Implementing Guide to provide the model action plan and assists individual national development. International cooperation for the technical improvement and awareness cultivation is promoted. Examples in such national developments will be introduced and prospective technical/institutional prerequisite for nuclear forensics response framework will be studied.

Journal Articles

Round-robin $$^{230}$$Th-$$^{234}$$U age dating of bulk uranium for nuclear forensics

Gaffney, A.*; Hubert, A.*; Kinman, W. S.*; Magara, Masaaki; Okubo, Ayako; Pointurier, F.*; Schorzman, K. C.*; Steiner, R. E.*; Williams, R. W.*

Journal of Radioanalytical and Nuclear Chemistry, 307(3), p.2055 - 2060, 2016/03

 Times Cited Count:22 Percentile:89.8(Chemistry, Analytical)

In and inter-laboratory measurement comparison study, four laboratories (LLNL, LANL, CEA, JAEA) determined $$^{230}$$Th-$$^{234}$$U model ages of uranium certified reference material NBL U050 using isotope dilution mass spectrometry. The model dates determined by the participating laboratories range from 9 March 1956 to 19 October 1957, and are indistinguishable given the associated measurement uncertainties. These model ages are concordant with to slightly older than the known production age of NBL U050, indicating unsufficient purification of U050.

Oral presentation

Oral presentation

Age-dating of single particle of uranium standard material for nuclear forensics and safeguards

Okubo, Ayako; Esaka, Fumitaka; Magara, Masaaki; Shinohara, Nobuo

no journal, , 

To elucidate the final purification date of uranium material namely age-dating is important subject on nuclear forensic analysis. Age-dating of uranium using $$^{234}$$U-$$^{230}$$Th nuclide pair was established in the field of geochemical science, and has been applied for nuclear forensics. Recently, safeguard analysis also demand age-dating of uranium materials. In order to measure a small amount of $$^{230}$$Th by ICP-MS, anion exchange column separation is commonly conducted to eliminate U tailing effect. However, column separation step could raise procedural blank of $$^{230}$$Th. In contrast, TIMS can separately ionize U and Th in filament heating step using the difference of optical ionization temperature of these elements. We developed analytical method for age-dating of single particle uranium material by TIMS.

Oral presentation

Technology and development for nuclear forensics; Result of ITWG collaborative materials exercise

Okubo, Ayako; Shinohara, Nobuo; Toda, Nobufumi; Kataoka, Osamu; Matsumoto, Tetsuya

no journal, , 

no abstracts in English

Oral presentation

Nuclear forensics and radiochemistry

Shinohara, Nobuo; Kimura, Yoshiki; Okubo, Ayako

no journal, , 

Nuclear forensics is the analysis of intercepted illicit nuclear or radioactive material and any associated material to provide evidence for nuclear attribution by determining origin, history, transit routes and purpose involving such material. Because the nuclear forensics methodologies provide hints of the origin of the nuclear materials used in illegal dealings or nuclear terrorism, it contributes to identify and indict offenders, hence to enhance deterrent effect against such terrorism. In the 59th Symposium on Radiochemistry, the results of research and development of fundamental nuclear forensics technologies (analysis of isotopic composition, impurity analysis, age dating of nuclear material, particle shape analysis by electron microscope, and nuclear forensics library) performed in Japan Atomic Energy Agency are reported. Japan's capability and the role of radiochemistry on nuclear forensics are also discussed in the Symposium.

Oral presentation

Development of uranium age-dating using $$^{234}$$Th/$$^{230}$$Th ratios

Okubo, Ayako; Shinohara, Nobuo; Magara, Masaaki

no journal, , 

The uranium age-dating is a nuclear forensics analysis techniques, by measuring the $$^{230}$$Th / $$^{234}$$U isotope ratio in uranium sample, to estimate the elapsed time from being separated and purified. We have determined $$^{230}$$Th and $$^{234}$$U using isotope dilution mass spectrometry method, it has conducted for uranium age-dating. Act to perform the isotope analysis after the addition a known quantity of the isotope (spike) to the sample, after spiking, analytical sample is assumed to be in the state of isotopic equilibrium. However, the samples which have complex speciation of uranium and thorium are analyzed, may not sufficiently reach to the state of isotopic equilibrium has been suggested from the experimental results. In this study, without the addition of a spike, from the measurement results of the uranium isotope ratios and thorium isotope ratio in the sample, it was investigated a method for calculating the $$^{230}$$Th / $$^{234}$$U isotope ratio. The state of radioactive equilibrium between $$^{238}$$U and $$^{234}$$Th in the sample was utilized in the $$^{234}$$Th / $$^{230}$$Th method. The $$^{230}$$Th / $$^{234}$$U ratio was calculated using measured $$^{234}$$Th / $$^{230}$$Th isotope ratio, $$^{234}$$U / $$^{238}$$U isotope ratio and $$^{234}$$Th / $$^{238}$$U ratio in the radioactive equilibrium.

Oral presentation

Readiness for nuclear terrorism; Nuclear forensics framework in advanced nations

Tamai, Hiroshi; Kimura, Yoshiki; Okubo, Ayako; Shinohara, Nobuo; Tomikawa, Hirofumi

no journal, , 

Nuclear forensics is effective measure for strengthening nuclear security through the analysis of origin and characteristics of nuclear materials or radio-isotopes collected at the crime scene inspections. In the development of nuclear forensics laboratory/library, "Chain of Custody" should be kept in mind on the view point of juridical process. Each nation should develop own national response plan to stipulate the framework for integrated nuclear forensics activities. Good practices for stipulating national frameworks for nuclear forensics are investigated in advancing nations such as US, EU and Canada. Issues and measures are proposed aiming at improving its framework.

Oral presentation

Development of nuclear forensics capabilities in Japan; New age-dating method

Okubo, Ayako; Shinohara, Nobuo; Umino, Yuji; Hara, Mikiya

no journal, , 

Oral presentation

Oral presentation

Joint validation of the in-situ uranium age dating method

Okubo, Ayako; Mayer, K.*

no journal, , 

Under the collaboration between EC-JRC and JAEA, the in-situ age dating method was subject to joint validation, and six different uranium materialswere used for this purpose. The age dating result by in-situ isotope method was consistent with known production dates of the respective samples. The uncertainty evaluation according to GUM for the in-situ isotope method indicates that the measured $$^{234}$$Th/$$^{230}$$Th ratio provides the highest contribution. The accuracy of in-situ isotope method can be improved by higher precision in $$^{234}$$Th/$$^{230}$$Th measurement.

Oral presentation

JAEA's initial efforts on buildup of nuclear forensics capability in Asian countries

Tomikawa, Hirofumi; Kimura, Yoshiki; Okubo, Ayako

no journal, , 

Oral presentation

Joint sample analysis on selected uranium ore concentrates and nuclear forensics library exercise

Kips, R.*; Lindvall, R.*; Marks, N.*; Gluschenko, V.*; Okubo, Ayako; Szeles, E.*

no journal, , 

Oral presentation

Development of nuclear security technologies for response on material out of regulatory control event and nuclear forensics activities in Japan

Kimura, Yoshiki; Tsuchiya, Kenichi*; Okubo, Ayako*; Tanabe, Kosuke*; Kakuda, Hidetoshi*; Akiba, Norimitsu*; Tomikawa, Hirofumi

no journal, , 

27 (Records 1-20 displayed on this page)